Synthesis of Some Glycosylated Derivatives of 2-Deoxy-2-fluoro-β-laminaribiosyl Fluoride: Another Success for Glycosynthases

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Abstract

The synthesis of 4,6-di-O-acetyl-2-deoxy-2-fluoro-3-O-(tetra-O-acetyl-beta-D-glucopyranosyl)-beta-D-glucosyl fluoride is described. Upon deacetylation and treatment with alpha-D-glucopyranosyl fluoride in the presence of a glycosynthase, three products, all 2-deoxy-2-fluoro-beta-glycosyl fluorides, could be isolated: a trisaccharide, a tetrasaccharide, and a pentasaccharide. An attempt to convert a trisaccharide glycal into a related difluoride, employing Selectfluor, is also reported.
Original languageEnglish
Pages (from-to)83-88
JournalAustralian Journal of Chemistry: an international journal for chemical science
Volume60
Issue number1
DOIs
Publication statusPublished - 2007

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