TY - JOUR
T1 - Micro Eddy Current Facilitated by Screwed MoS2 Structure for Enhanced Hydrogen Evolution Reaction
AU - Su, Meixia
AU - Zhou, Wenda
AU - Liu, Lin
AU - Chen, Mingyue
AU - Jiang, Zhenzhen
AU - Luo, Xingfang
AU - Yang, Yong
AU - Yu, Ting
AU - Lei, Wen
AU - Yuan, Cailei
PY - 2022/5/25
Y1 - 2022/5/25
N2 - Eddy current is a magnetic field effect generated in alternating magnetic field (AMF), which could trigger continuous local heating, reducing the energy consumption without impairing the life of the catalyst or reactor. Unfortunately, the investigation of eddy current effect on transition metal disulfides (TMDs) electrocatalysis is still in its infancy, and its actual electrocatalytic applications has been impeded by the multilayered structure of traditional layered TMDs. Typically, the step pyramid MoS2, with a layer-by-layer stacking structure just like the silicon steel plate in the transformer, showing an inevitable interlayer potential barrier will suppress the generation of eddy current and cause low efficiency of magnetic heating. In this work, the designed screw pyramid MoS2 can facilitate the formation of micro eddy current and maximize utilization of magnetic heating to boost electrocatalytic activity, benefiting from its eliminated interlayer potential barrier. This work provides a new thinking for the design of field-assisted electrocatalytic reactions and development of the advanced catalyst technology.
AB - Eddy current is a magnetic field effect generated in alternating magnetic field (AMF), which could trigger continuous local heating, reducing the energy consumption without impairing the life of the catalyst or reactor. Unfortunately, the investigation of eddy current effect on transition metal disulfides (TMDs) electrocatalysis is still in its infancy, and its actual electrocatalytic applications has been impeded by the multilayered structure of traditional layered TMDs. Typically, the step pyramid MoS2, with a layer-by-layer stacking structure just like the silicon steel plate in the transformer, showing an inevitable interlayer potential barrier will suppress the generation of eddy current and cause low efficiency of magnetic heating. In this work, the designed screw pyramid MoS2 can facilitate the formation of micro eddy current and maximize utilization of magnetic heating to boost electrocatalytic activity, benefiting from its eliminated interlayer potential barrier. This work provides a new thinking for the design of field-assisted electrocatalytic reactions and development of the advanced catalyst technology.
KW - alternating magnetic field
KW - hydrogen evolution reaction
KW - micro eddy current
UR - https://www.scopus.com/pages/publications/85125135849
U2 - 10.1002/adfm.202111067
DO - 10.1002/adfm.202111067
M3 - Article
AN - SCOPUS:85125135849
SN - 1616-301X
VL - 32
JO - Advanced Functional Materials
JF - Advanced Functional Materials
IS - 22
M1 - 2111067
ER -