TY - JOUR
T1 - Catalytic performance of coal char for the methane reforming process
AU - He, T.
AU - Sun, Z.
AU - Wu, J.
AU - Xu, Z.
AU - Zhang, Dongke
AU - Han, D.
PY - 2014
Y1 - 2014
N2 - © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. A new concept of combined coal gasification and methane reforming in a single reactor was proposed as an alternative path for syngas production using coal and coalbed methane. Here, the results of this process are summarized. The experimental work was carried out in a fixed-bed reactor. Methane cracking, CO2/steam reforming of methane over coal char, and the effects of chars made from different types of parent coal on methane conversion were examined. The catalytic effect of coal char on methane cracking and reforming increased with decreasing coalification degree. A synergistic effect was observed in that, while the coal char catalyzed the methane reforming reactions, gasification of the coal char took place simultaneously, which counter-balanced the deposition of carbon especially for the methane-steam-char system.
AB - © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. A new concept of combined coal gasification and methane reforming in a single reactor was proposed as an alternative path for syngas production using coal and coalbed methane. Here, the results of this process are summarized. The experimental work was carried out in a fixed-bed reactor. Methane cracking, CO2/steam reforming of methane over coal char, and the effects of chars made from different types of parent coal on methane conversion were examined. The catalytic effect of coal char on methane cracking and reforming increased with decreasing coalification degree. A synergistic effect was observed in that, while the coal char catalyzed the methane reforming reactions, gasification of the coal char took place simultaneously, which counter-balanced the deposition of carbon especially for the methane-steam-char system.
U2 - 10.1002/ceat.201400124
DO - 10.1002/ceat.201400124
M3 - Article
VL - 38
SP - 68
EP - 74
JO - Chemical Engineering and Technology
JF - Chemical Engineering and Technology
SN - 0930-7516
IS - 1
ER -